Gonoskov I, Gräfe S (2021)
Publication Type: Journal article
Publication year: 2021
Book Volume: 154
Article Number: 234106
Journal Issue: 23
DOI: 10.1063/5.0048930
We propose a novel general approximation to transform and simplify the description of a complex fully quantized system describing the interacting light and matter. The method has some similarities to the time-dependent Born-Oppenheimer approach: we consider a quantum description of light rather than of nuclei and follow a similar separation procedure. Our approximation allows us to obtain a decoupled system for the light-excited matter and "dressed"light connected parametrically. With these equations at hand, we study how intense light as a quantum state is affected due to the back-action of the interacting matter. We discuss and demonstrate the possibility of the light-mode entanglement and nonclassical light generation during the interaction.
APA:
Gonoskov, I., & Gräfe, S. (2021). Light matter quantum dynamics of complex laser-driven systems. Journal of Chemical Physics, 154(23). https://doi.org/10.1063/5.0048930
MLA:
Gonoskov, Ivan, and Stefanie Gräfe. "Light matter quantum dynamics of complex laser-driven systems." Journal of Chemical Physics 154.23 (2021).
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