Ultrafast control of spin-orbital separation probed with time-resolved resonant inelastic x-ray scattering

Müller A, Grandi F, Eckstein M (2022)


Publication Type: Journal article

Publication year: 2022

Journal

Book Volume: 106

Article Number: L121107

Journal Issue: 12

DOI: 10.1103/PhysRevB.106.L121107

Abstract

Quasi-one-dimensional systems exhibit many-body effects elusive in higher dimensions. A prime example is spin-orbital separation, which has been measured by resonant inelastic x-ray scattering (RIXS) in Sr2CuO3. Here, we theoretically analyze the time-resolved RIXS spectrum of Sr2CuO3 under the action of a time-dependent electric field. We show that the external field can reversibly modify the parameters in the effective t-J model used to describe spinon and orbiton dynamics in the material. For strong driving amplitudes, we find that the spectrum changes qualitatively as a result of reversing the relative spinon to orbiton velocity. The analysis shows that in general, the spin-orbital dynamics in Mott insulators in combination with time-resolved RIXS should provide a suitable platform to explore the reversible control of many-body physics in the solid with strong laser fields.

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How to cite

APA:

Müller, A., Grandi, F., & Eckstein, M. (2022). Ultrafast control of spin-orbital separation probed with time-resolved resonant inelastic x-ray scattering. Physical Review B, 106(12). https://doi.org/10.1103/PhysRevB.106.L121107

MLA:

Müller, Aaron, Francesco Grandi, and Martin Eckstein. "Ultrafast control of spin-orbital separation probed with time-resolved resonant inelastic x-ray scattering." Physical Review B 106.12 (2022).

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