Photoinduced metallization of excitonic insulators

Ejima S, Lange F, Fehske H (2022)


Publication Type: Journal article

Publication year: 2022

Journal

Book Volume: 105

Article Number: 245126

Journal Issue: 24

DOI: 10.1103/PhysRevB.105.245126

Abstract

Utilizing the time-dependent density-matrix renormalization-group technique, we numerically prove photoinduced pairing states in the extended Falicov-Kimball model (EFKM) at half-filling, both with and without internal SU(2) symmetry. In the time-dependent photoemission spectra, an extra band appears above the Fermi energy after pulse irradiation, indicating an insulator-to-metal transition. Even in the absence of the SU(2) structure, the pair correlations are enhanced during the pump, and afterwards they decrease over time. This implies the possible metallization of Ta2NiSe5, a strong candidate for an excitonic insulator material, for which the EFKM is considered to be the minimal theoretical model. Simulating the photoemission with optimized pulse parameters, we demonstrate a photoinduced quantum phase transition, in accord with recent findings in time- and angle-resolved photoemission spectroscopy experiments on Ta2NiSe5.

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How to cite

APA:

Ejima, S., Lange, F., & Fehske, H. (2022). Photoinduced metallization of excitonic insulators. Physical Review B, 105(24). https://dx.doi.org/10.1103/PhysRevB.105.245126

MLA:

Ejima, Satoshi, Florian Lange, and Holger Fehske. "Photoinduced metallization of excitonic insulators." Physical Review B 105.24 (2022).

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