Fortunato GV, Pizzutilo E, Mingers AM, Kasian O, Chereyko S, Cardoso ESF, Mayrhofer K, Maia G, Ledendecker M (2018)
Publication Status: Published
Publication Type: Journal article
Publication year: 2018
Publisher: AMER CHEMICAL SOC
Book Volume: 122
Pages Range: 15878-15885
Journal Issue: 28
A successful market introduction of electrocatalytically produced hydrogen peroxide (H2O2) requires catalysts that are highly selective, active, and economically suitable. Here, we present important insights into tuning the selectivity toward H2O2 and elaborate on the opportunities opened for high catalytic performance. Especially the metal loading, the accompanied interparticle distance, and catalyst support interaction were identified as key contributors for high selectivity and activity. We focused on the design of model catalysts with different Pd loadings and distinct interparticle distances and their dependency on the selectivity toward H2O2. The gained understandings can be used as guidelines for the development of highly active and selective catalysts while simultaneously reducing the noble metal loading and the associated costs.
APA:
Fortunato, G.V., Pizzutilo, E., Mingers, A.M., Kasian, O., Chereyko, S., Cardoso, E.S.F.,... Ledendecker, M. (2018). Impact of Palladium Loading and Interparticle Distance on the Selectivity for the Oxygen Reduction Reaction toward Hydrogen Peroxide. Journal of Physical Chemistry C, 122(28), 15878-15885. https://doi.org/10.1021/acs.jpcc.8b04262
MLA:
Fortunato, Guilherme V., et al. "Impact of Palladium Loading and Interparticle Distance on the Selectivity for the Oxygen Reduction Reaction toward Hydrogen Peroxide." Journal of Physical Chemistry C 122.28 (2018): 15878-15885.
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