Nanofacet-resolved CO oxidation kinetics on alumina- supported Pd particles

Libuda J (2002)


Publication Status: Published

Publication Type: Journal article

Publication year: 2002

Journal

Publisher: ELSEVIER SCIENCE BV

Book Volume: 354

Pages Range: 403-408

Journal Issue: 5-6

Abstract

Employing a multi-molecular-beam approach, we have measured the angular distribution of CO, molecules formed during CO oxidation under steady-state conditions on well oriented and shaped nm-sized Pd crystallites grown on an ordered alumina film. The experiment is combined with kinetic Monte Carlo simulations based on a realistic structural model. The results obtained allow us (i) to differentiate between local reaction rates on the particle nanofacets and (ii) to conclude that oxygen diffusion on and between the (111) facets is rapid compared to reaction. (C) 2002 Elsevier Science B.V. All rights reserved.

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How to cite

APA:

Libuda, J. (2002). Nanofacet-resolved CO oxidation kinetics on alumina- supported Pd particles. Chemical Physics Letters, 354(5-6), 403-408.

MLA:

Libuda, Jörg. "Nanofacet-resolved CO oxidation kinetics on alumina- supported Pd particles." Chemical Physics Letters 354.5-6 (2002): 403-408.

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